The three manual uninstall parts
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Step 1
Revert root patches
Open OCLP, go to Post Install Root Patch, and choose Revert Root Patches. Monterey and later support snapshot reversion; Big Sur may require reinstall.
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Step 2
Remove the application
Use the uninstaller package from the project releases page to remove the app, LaunchAgent, and PrivilegedHelperTool.
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Step 3
Remove OpenCore from EFI
Mount the EFI partition and remove EFI/OC and System folders. Do not delete the whole EFI folder because it may contain Windows or Linux boot files.
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Step 4
Reset NVRAM
Reset NVRAM after removing OpenCore to return boot variables to a cleaner state.
Before removing the bootloader
The uninstall docs warn that after removing OpenCore, your Mac may no longer boot newer patched macOS and may show the prohibited symbol.
Prepare a bootable USB drive with OpenCore or a natively supported macOS installer before removing the bootloader.